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Particulate emissions from IC engines associated with transient engine conditions are very important (similar to the legislated gaseous emissions). This is true both during real-world and test cycle driving. This paper describes an instrument for measuring the number of particles, and their spectral weighting, in the 5nm to 1000nm size range, with a time response of 200ms. This is achieved via an electrostatic classification technique, consisting of a diffusion charger followed by a multi-element, constant voltage, classifier. Conversion of the data to other metrics, such as mass, is also described. Results are presented from artificial test aerosols and from light and heavy duty diesel engines on standard test cycles.

The emission capability of an exhaust system tuned for improved engine performance from an in-line four-cylinder engine has been investigated. The exhaust system comprises two close-coupled catalysts; each located in separate exhaust streams and has been termed the 4-2 close-coupled catalysts (CCC) -1 system. It has been shown that, given equivalent total catalyst volume, this system configuration results in compromised high exhaust flow rate emissions performance compared with a single catalyst (4-1semi-CCC) system. This emissions performance deficit has been attributed to the effect of engine frequency flow pulsations, which result in relatively high peak space velocities in the 4-2CCC-1 system despite the mean space velocity being consistent. Engine-based AFR Bias Sweep tests suggest that hydrocarbon emissions are most strongly affected by this phenomenon. At lower exhaust flow rates, the difference in performance between the two systems is negligible.

Engines with reduced emissions and improved efficiency are of high interest for road transport. However, achieving these two goals is challenging and various concepts such as PFI/DI/HCCI/PCCI are explored by engine manufacturers. The computational fluid dynamics is becoming an integral part of modern engine development programme because this method provides access to in-cylinder flow and thermo-chemical processes to develop a closer understanding to tailor tumble and swirling motions to construct green engines. The combustion modelling, its accuracy and robustness play a vital role in this. Out of many modelling methods proposed in the past flamelet based methods are quite attractive for SI engine application. In this study, FlaRe (Flamelets revised for physical consistencies) approach is used to simulate premixed combustion inside a gasoline PFI single-cylinder, four-stroke SI engine. This approach includes a parameter representing the effects of flame curvature on the burning rate.

This work presents turbulent premixed combustion modeling in spark ignition engines using G-equation based turbulent combustion model. In present study, a turbulent flame speed expression proposed and validated in recent years by two co-authors of this paper is applied to the combustion simulation of spark ignition engines. This turbulent flame speed expression has no adjustable parameters and its constants are closely tied to the physics of scalar mixing at small scales. Based on this flame speed expression, a minor modification is introduced in this paper considering the fact that the turbulent flame speed changes to laminar flame speed if there is no turbulence. This modified turbulent flame speed expression is implemented into Ford in-house CFD code MESIM (multi-dimensional engine simulation), and is validated extensively.

A dual-fuel approach to control combustion in HCCI engine is investigated in this work. This approach involves controlling the combustion heat release rate by adjusting fuel reactivity according to the conditions inside the cylinder. Experiments were performed on a single-cylinder research engine fueled with different ratios of primary reference fuels and operated at different speed and load conditions, and results from these experiments showed a clear potential for the approach to expand the HCCI engine operation window. Such potential is further demonstrated dynamically using an optimized stochastic reactor model integrated within a MATLAB code that simulates HCCI multi-cycle operation and closed-loop control of fuel ratio. The model, which utilizes a reduced PRF mechanism, was optimized using a multi-objective genetic algorithm and then compared to a wide range of engine data.

A multi-objective optimization scheme based on stochastic global search is developed and used to examine the performance of an HCCI model containing a reduced chemical kinetic mechanism, and to study interrelations among different model responses. A stochastic reactor model of an HCCI engine is used in this study, and dedicated HCCI engine experiments are performed to provide reference for the optimization. The results revealed conflicting trends among objectives normally used in mechanism optimization, such as ignition delay and engine cylinder pressure history, indicating that a single best combination of optimization variables for these objectives did not exist. This implies that optimizing chemical mechanisms to maintain universal predictivity across such conflicting responses will only yield a predictivity tradeoff. It also implies that careful selection of optimization objectives increases the likelihood of better predictivity for these objectives.

An on-board version of a fast response chemiluminsescence analyzer with a 3-millisecond response time enables the recording of high temporal resolution transient NOx emissions during cold start and pull-away, gear changes, speed bumps and other real world transient conditions. Tests were initially performed on a 1.6 litre turbo GDI vehicle before comparison with a diesel vehicle. The data has been correlated with on-board engine data available from the vehicle’s electronic control unit to study the underlying causes of these short-duration events. Exhaust gas was generally sampled from downstream of the after treatment system but before the silencer (muffler) to preserve all high frequency detail and to allow accurate integration of pollutant concentration and engine exhaust mass flow.

Results from a large set of HCCI experiments performed on a single-cylinder research engine fueled with different mixtures of iso-octane and n-heptane are presented and discussed in this paper. The experiments are designed to scrutinize fuel reactivity effects on the operating range of an HCCI engine. The fuel effects on upper and lower operating limits are measured respectively by the maximum pressure rise rate inside the cylinder and the stability of engine operation as determined by cycle-to-cycle variations in IMEP. Another set of experiments that examine the intake air heating effects on HCCI engine performance, exhaust emissions and operating envelopes is also presented. The effects of fuel reactivity and intake air heating on the HCCI ranges are demonstrated by constructing the operating envelopes for the different test fuels and intake temperatures.

An accurate prediction of residual burned gas within the combustion chamber is important to quantify for development of modern engines, especially so for those with internally recycled burned gases and HCCI operations. A wall-guided GDI engine has been fitted with an in-cylinder sampling probe attached to a fast response NDIR analyser to measure in-situ the cycle-by-cycle trapped residual gas. The results have been compared with a model which predicts the trapped residual gas fraction based on heat release rate calculated from the cylinder pressure data and other factors. The inlet and exhaust valve timings were varied to produce a range of Residual Gas Fraction (RGF) conditions and the results were compared between the actual measured CO2 values and those predicted by the model, which shows that the RGF value derived from the exhaust gas temperature and pressure measurement at EVC is consistently overestimated by 5% over those based on the CO2 concentrations.

The gaseous and particulate emissions from a diesel passenger car have been studied during cold start and Diesel Particulate Filter (DPF) regeneration events occurring during the New European Drive Cycle (NEDC). During the initial phase of the cycle, Diesel Oxidation Catalyst (DOC) light-off was seen to be highly dynamic with catalyst efficiency changing dramatically with changes in catalyst temperature. Accumulation mode particulate emissions were sampled directly from the exhaust after the DPF. From cold start with a clean (regenerated) DPF, accumulation mode particle emissions were seen to be very much higher than those from a loaded DPF. This accumulation mode slip lasted only approximately 200 seconds. During regeneration of the DPF, the oxidation of trapped soot was associated with a large tailpipe emission of nucleation mode particles.

We numerically simulate a Homogeneous Charge Compression Ignition (HCCI) engine fuelled with a blend of ethanol and diethyl ether by means of a stochastic reactor model (SRM). A 1D CFD code is employed to calculate gas flow through the engine, whilst the SRM accounts for combustion and convective heat transfer. The results of our simulations are compared to experimental measurements obtained using a Caterpillar CAT3401 single-cylinder Diesel engine modified for HCCI operation. We consider emissions of CO, CO2 and unburnt hydrocarbons as functions of the crank angle at 50% heat release. In addition, we establish the dependence of ignition timing, combustion duration, and emissions on the mixture ratio of the two fuel components. Good qualitative agreement is found between our computations and the available experimental data.

Flamelet modelling of premixed turbulent combustion can be applied to spark-ignition engine combustion. To address and validate several modelling criteria, two measurement techniques are used in a burner flame to study the interaction between turbulent flowfields and combustion for subsequent application to engine combustion. Particle Image Velocimetry and Light Sheet Tomography are used together to measure conditional velocities simultaneously in reactant and product mixtures. Correlations of velocity and reaction scalar fluctuations indicate that counter-gradient turbulent diffusion must be accounted for when modelling this flowfield. Comparisons of spatial averaging of instantaneous and ensemble-averaged data are made and the application of similar techniques to engine combustion is discussed.

A fast response NO detector has been developed to study fast transient emissions from internal combustion engines. The device combines the standard ChemiLuminescence Detector (CLD) measurement technique used in conventional NO detectors with the rapid sampling system of an existing Fast Flame Ionisation Detector (FFID) hydrocarbon detector. The 10-90% response time of the fast NO detector is approximately 3 milliseconds and enables resolution of transient NO concentration within individual engine cycles. Both the fast NO and fast HC detectors were fitted in the exhaust port of a firing SI engine. With the probe tips at the same position, simultaneous fast transient NO and HC concentration data have been recorded during steady state and transient engine load conditions. Cycle-by-cycle NO concentration, HC concentration, and cylinder pressure are compared and features of the transient NO and HC concentration are discussed.

Using a novel, high frequency response FID unit, hydrocarbon measurements in the spark plug gap of a firing gasoline engine have been made. These measurements have been correlated with the pressure development, and a significant correlation was found. The method described can be used on any engine fitted with a modified sparking plug.

Experiments were performed to measure the number-weighted particle size distributions emitted from a gasoline direct injection (GDI) engine. Measurements were made on a late model vehicle equipped with a direct injection spark ignition engine. The vehicle was placed on a chassis dynamometer, which was used to load the engine to road load at five different vehicle speeds ranging from 15 - 100 km/hr. Dilution of the exhaust aerosol was carried out using a two-stage dilution system in which the first stage dilution occurs as a free jet. Particle size distributions were measured using a TSI 3934 scanning mobility particle sizer. Generally speaking, the presence of the additives did not have a strong, consistent influence on the particle emissions from this engine. The polyether amine demonstrated a reduction in particle number concentration as compared to unadditized base fuel.

The development and optimisation of an ultra-fast response chemiluminescence NOx analyser, equipped with a high temperature stainless steel, nitrogen dioxide (NO2) to nitric oxide (NO) converter, for the transient measurement of the NOx (NO + NO2) content of automotive emissions is described. Conventional analysers routinely used to measure NOx in automotive exhaust utilise chemiluminescence detection (CLD). Ultra-fast time-scale analysis using CLD, however, has traditionally been hindered by the slow conversion of NO2 to NO. The converter and technology used in the instrument described herein enables a 10-90% response time of less than 10 ms. Following optimisation in the laboratory, the fast response CLD NOx analyser was evaluated for raw exhaust sampling of port fuel injected (PFI) gasoline and diesel vehicles.

A turbulent combustion model is described for SI engines with large variations in mixture strength. The model is for a single gas phase fluid at high Reynolds number and treats combustion in the laminar flamelet regime, which is characterized by high Damkholer and low Karlovitz numbers. An assumed probability density function (pdf) approach is used to extract expressions for mean quantities of interest, which are parameterized on the progress variable and mixture fraction variables. A double delta function pdf is used for the reaction progress variable and a beta function pdf is used for the mixture fraction. The reaction rate term in the progress variable equation is closed using an algebraic expression, which incorporates the effects of mixture strength, pressure and temperature on laminar flame speed. The model is implemented in two versions of a Computational Fluid Dynamics (CFD) code.

A fast response sensor for measuring carbon dioxide concentration has been developed for laboratory research and tested on a spark ignition engine. The sensor uses the well known infra-red absorption technique with a miniaturized detection system and short capillary sampling tubes, giving a time constant of approximately 5 milliseconds; this is sufficiently fast to observe changes in CO2 levels on a cycle-by-cycle basis under normal operating conditions. The sensor is easily located in the exhaust system and operates continuously. The sensor was tested on a standard production four cylinder spark-ignition engine to observe changes in CO2 concentration in exhaust gas under steady state and transient operating conditions. The processed sensor signal was compared to a standard air-to-fuel ratio (AFR) sensor in the exhaust stream and the results are presented here. The high frequency response CO2 measurements give new insights into both engine and catalyst transient operation.

Experiments were performed to measure the average and time-resolved particle number emissions and number-weighted particle size distributions from a gasoline direct injection (GDI) engine. Measurements were made on a late model vehicle equipped with a direct injection spark ignition engine. The vehicle was placed on a chassis dynamometer, which was used to load the engine to road load at five different vehicle speeds ranging from 13 - 90 km/hr. Particle number emissions were measured using a TSI 3020 condensation nucleus counter, and size distributions were measured using a TSI 3934 scanning mobility particle sizer. Average polydisperse number concentration was found to increase from 1.1 × 108 particles/cm3 at 13 km/hr to 2.8 × 108 particles/cm3 at 70 km/hr. Under a closed-loop, stoichiometric homogeneous charge operating mode at 90 km/hr, number emissions fell to 9.3 × 107 particles/cm3 (at all other operating conditions, the engine was in a lean stratified charge operating mode).

A method for improving three-way catalyst (TWC) performance by superimposing a low frequency lean air-to-fuel ratio (AFR)bias perturbation onto the standard AFR oscillations is described. This observation of Catalyst Regeneration (CatRegen) has been attributed to a reactivation of poisoned precious metal sites on the catalyst surface. Preliminary tests under steady-state conditions show that there is a gradual reduction in TWC activity for NOx after a lean-rich transition, suggesting a temporary poisoning of the active precious metal sites on the TWC under rich conditions. This deactivation can be prevented by periodically exposing the catalyst to lean exhaust gas; which has led to the development of the CatRegen system.